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High-yield bottom-up synthesis of 2D metal-organic frameworks and their derived ultrathin carbon nanosheets for energy storage

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成果类型:
期刊论文
作者:
Zhao, Kuangmin;Liu, Suqin*;Ye, Guanying;Gan, Qingmeng;Zhou, Zhi;...
通讯作者:
Liu, Suqin;He, Zhen
作者机构:
[Gan, Qingmeng; He, Zhen; Liu, Suqin; Ye, Guanying; He, Z; Zhao, Kuangmin] Cent S Univ, Coll Chem & Chem Engn, Changsha 410083, Hunan, Peoples R China.
[Gan, Qingmeng; Ye, Guanying; Zhao, Kuangmin] Cent S Univ, Innovat Base Energy & Chem Mat Grad Students Trai, Changsha 410083, Hunan, Peoples R China.
[Zhou, Zhi] Hunan Agr Univ, Sci Coll, Changsha 410128, Hunan, Peoples R China.
通讯机构:
[Liu, SQ; He, Z] C
Cent S Univ, Coll Chem & Chem Engn, Changsha 410083, Hunan, Peoples R China.
语种:
英文
期刊:
Journal of Materials Chemistry A
ISSN:
2050-7488
年:
2018
卷:
6
期:
5
页码:
2166-2175
基金类别:
This work was supported by the National Natural Science Foundation of China (grant nos. 51372278, U1507106, and 21303270), the Hunan Provincial Science and Technology Plan Project, China (grant no. 2017TP1001), and the Innovation-Driven Project of Central South University (grant no. 2016CXS031).
机构署名:
本校为其他机构
院系归属:
理学院
摘要:
Two-dimensional (2D) metal-organic frameworks (MOFs) have been considered as promising precursors for the synthesis of 2D carbon materials for energy storage. However, the high costs and low yields of the synthetic methods for 2D MOFs are major obstacles for the preparation of 2D carbon materials from 2D MOFs. Herein, we report a facile and low-cost bottom-up synthesis of ultrathin Zn(bim)(OAc) MOF nanosheets (with a thickness of ∼5 nm and a high yield of ∼65%) and their derived N-doped porous ultrathin (2.5 ± 0.8 nm) carbon nanosheets (UT-C...

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