Regulating Lithium Nucleation and Deposition via MOF-Derived Co@C-Modified Carbon Cloth for Stable Li Metal Anode

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成果类型：

期刊论文

作者：

Zhou, Ting;Shen, Jiadong;Wang, Zhuosen;Liu, Jun*;Hu, Renzong;...

通讯作者：

Liu, Jun;Yu, Yan

作者机构：

[Wang, Zhuosen; Hu, Renzong; Zhu, Min; Zhou, Ting; Shen, Jiadong; Liu, Jun; Ouyang, Liuzhang] South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Pulp & Paper Engn, Guangdong Prov Key Lab Adv Energy Storage Mat, Guangzhou 510641, Guangdong, Peoples R China.

[Feng, Yuezhan] Zhengzhou Univ, Minist Educ, Key Lab Mat Proc & Mold, Zhengzhou 450002, Peoples R China.

[Liu, Hui] Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

[Yu, Yan] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Dept Mat Sci & Engn, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.

[Yu, Yan] Chinese Acad Sci, Dalian Natl Lab Clean Energy DNL, Dalian 116023, Liaoning, Peoples R China.

通讯机构：

[Liu, Jun] S

[Yu, Yan] U

[Yu, Yan] C

South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Pulp & Paper Engn, Guangdong Prov Key Lab Adv Energy Storage Mat, Guangzhou 510641, Guangdong, Peoples R China.

Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Dept Mat Sci & Engn, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.

语种：

英文

关键词：

adsorption energy;Li metal anodes;lithiophilic frameworks;metal Co;self-supported arrays

期刊：

Advanced Functional Materials

ISSN：

1616-301X

年：

2020

卷：

期：

页码：

1909159-

DOI：

10.1002/adfm.201909159

基金类别：

National Key R&D Research Program of China [2018YFB0905400]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China [51771076, 51872277, 51925207, U1910210]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [WK2060140026]; DNL cooperation Fund, CAS [DNL180310]; Innovative Research Groups of the National Natural Science Foundation of ChinaNational Natural Science Foundation of China [NSFC51621001]; "1000 plan" from Chinese Government; Guangdong "Pearl River Talents Plan" [2017GC010218]; Guangzhou Science and Technology Plan Projects [201804010104]

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本校为其他机构

院系归属：

理学院

摘要：

Lithium metal is an exciting anode candidate with extra high theoretical specific capacity for new high-energy rechargeable batteries. However, uncontrolled Li deposition and an unsteady solid electrolyte interface seriously obstruct the commercial application of Li anodes in Li metal batteries. Herein, 3D carbon cloth (CC) supporting N-doped carbon (CN) nanosheet arrays embedded with tiny Co nanoparticles (CC@CN-Co) are employed as a lithiophilic framework to regulate homogenous Li nucleation/growth behavior in a working Li metal anode. The em...

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Regulating Lithium Nucleation and Deposition via MOF-Derived Co@C-Modified Carbon Cloth for Stable Li Metal Anode

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