Self-assembled sulphur doped carbon nitride for photocatalytic water reforming of methanol

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成果类型：

期刊论文

作者：

Wang, Hui;Thangamuthu, Madasamy;Wu, Zhibin;Yang, Jianlong;Yuan, Hongzhao;...

通讯作者：

Tang, Junwang(junwang.tang@ucl.ac.uk)

作者机构：

[Thangamuthu, Madasamy; Wang, Hui; Tang, Junwang] UCL, Dept Chem Engn, London WC1E 7JE, England.

[Wu, Zhibin] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.

[Yang, Jianlong] Northwest Univ, Coll Chem & Mat Sci, Key Lab Synthet, Energy & Catalysis Hub, Xi'an 710127, Peoples R China.

[Yuan, Hongzhao] Chinese Acad Sci, Inst Subtrop Agr, Key Lab Agroecol Proc Subtrop Reg, Changsha 410125, Hunan, Peoples R China.

[Yang, Jianlong] Northwest Univ, Coll Chem & Mat Sci, Nat Funct Mol Chem Minist Educ, Energy & Catalysis Hub, Xi'an 710127, Peoples R China.

通讯机构：

[Junwang Tang] D

Department of Chemical Engineering, University College London, London WC1E 7JE, UK

语种：

英文

关键词：

C-S-H bonds;Doped graphitic carbon nitride;H2 production;High stability;Photocatalysis;Water reforming of methanol

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2022

卷：

445

页码：

136790

DOI：

10.1016/j.cej.2022.136790

基金类别：

All authors thank UK EPSRC (EP/S018204/2), Leverhulme Trust (RPG-2017-122), Royal Society Newton Advanced Fellowship grant (NAF\R1\191163), Royal Society International Exchange Scheme (IEC\NSFC\170342) and Royal Society Leverhulme Trust Senior Research Fellowship (SRF\R1\21000153).

机构署名：

本校为其他机构

院系归属：

资源环境学院

摘要：

The ability to effectively harness and store renewable solar energy in chemical forms, e.g., methanol has been widely recognised as a promising and sustainable strategy for H2 storage. Though traditional steam reforming of methanol enables effective H2 release from methanol and water, the harsh operating conditions result in high energy consumption and CO by-product. To minimize CO emission and maximise H2 production, photocatalytic liquid water reforming of methanol has been developed to produce H2 by sulphur doped graphitic carbon nitride (SC...

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Self-assembled sulphur doped carbon nitride for photocatalytic water reforming of methanol

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