Robust Electrodes with Maximized Spatial Catalysis for Vanadium Redox Flow Batteries

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成果类型：

期刊论文

作者：

Sheng, Hang;Ma, Qiang;Yu, Jin-Gang;Zhang, Xu-Dong;Zhang, Wei;...

通讯作者：

Wu, Xiongwei;Zeng, Xian-Xiang;Guo, Yu-Guo

作者机构：

[Ma, Qiang; Sheng, Hang; Zhang, Wei; Wu, Xiongwei; Wu, XW; Zeng, Xian-Xiang] Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

[Ma, Qiang; Sheng, Hang; Zhang, Xu-Dong; Yin, Ya-Xia; Guo, Yu-Guo] Chinese Acad Sci, CAS Res Educ Ctr Excellence Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Beijing 100190, Peoples R China.

[Yu, Jin-Gang] Cent S Univ, Hunan Prov Key Lab Efficient & Clean Utilizat Man, Coll Chem & Chem Engn, Changsha 410083, Hunan, Peoples R China.

通讯机构：

[Wu, XW; Zeng, XX] H

[Guo, Yu-Guo] C

Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

Chinese Acad Sci, CAS Res Educ Ctr Excellence Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Beijing 100190, Peoples R China.

语种：

英文

关键词：

electrocatalysis;vanadium redox flow battery;3D conducting network;electrode;energy efficiency

期刊：

ACS Applied Materials & Interfaces

ISSN：

1944-8244

年：

2018

卷：

期：

页码：

38922-38927

DOI：

10.1021/acsami.8b13778

基金类别：

Basic Science Center Project of the Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51788104]; National Key R&D Program of China [2016YFA0202500]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21773264, 51772301, 51803054]; Transformational Technologies for Clean Energy and Demonstration; Strategic Priority Research Program of the Chinese Academy of SciencesChinese Academy of Sciences [XDA21070300]

机构署名：

本校为第一且通讯机构

院系归属：

理学院

摘要：

Catalytic efficiency is a crucial index for electrodes in flow batteries, and tremendous efforts have been devoted to exploring catalysts with as many reaction zones as possible. Nevertheless, the space between the reaction sites, especially for interstitial space utilization, is usually ignored and challengeable to exploit owing to the balance between the catalytic efficiency and structural stability. Herein, a three-dimensional conducting network was constructed via a nitrogen-rich carbon film-bridged graphite felt framework (GF@N-C) to maxim...

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Robust Electrodes with Maximized Spatial Catalysis for Vanadium Redox Flow Batteries

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