Surface-wrinkle-modified graphite felt (GF) with abundant N and O is prefabricated by a hydrothermal method followed by calcination, and its surface morphology, elemental composition, and electrochemical properties are characterized by scanning electron microscopy, Raman spectroscopy, X-ray photoelectron spectroscopy, cyclic voltammetry, electrochemical impedance spectroscopy, and charge/discharge tests. The highly folded coating has excellent wettability, abundant catalytic sites, a fast ion-diffusion rate, ultralow interface transfer resistan...