Theoretical Investigation into Suitable Pore Sizes of Membranes for Vanadium Redox Flow Batteries

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成果类型：

期刊论文

作者：

Liu, Zaichun;Li, Ruilian;Chen, Jizhong;Wu, Xiongwei*;Zhang, Kai;...

通讯作者：

Wu, Xiongwei;Wu, Yuping;Holze, Rudolf

作者机构：

[Li, Ruilian; Liu, Zaichun; Yuan, Xinhai; Wu, Xiongwei; Mo, Jun; Wu, XW; Wu, Yuping; Zhang, Kai; Jiang, Hongmei] Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

[Liu, Zaichun; Wu, Yuping] Nanjing Tech Univ, Inst Electrochem Energy Storage, Sch Energy Sci & Engn, Nanjing 211816, Jiangsu, Peoples R China.

[Chen, Jizhong] State Key Lab Operat & Control Renewable Energy &, Beijing, Peoples R China.

[Wu, Xiongwei; Wu, XW; Wu, Yuping] Hunan Prov Yinfeng New Energy Co LTD, Changsha 410000, Hunan, Peoples R China.

[Holze, Rudolf] Tech Univ Chemnitz, Inst Chem, D-09107 Chemnitz, Germany.

通讯机构：

[Wu, XW; Wu, YP] H

[Wu, Yuping] N

[Holze, Rudolf] T

Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

Nanjing Tech Univ, Inst Electrochem Energy Storage, Sch Energy Sci & Engn, Nanjing 211816, Jiangsu, Peoples R China.

语种：

英文

关键词：

vanadium redox flow batteries;ion-exchange membranes;density functional calculations;pore size

期刊：

ChemElectroChem

ISSN：

2196-0216

年：

2017

卷：

期：

页码：

2184-2189

DOI：

10.1002/celc.201700244

基金类别：

National Materials Genome Project#&#&#2016YFB0700600 Distinguished Young Scientists Program of NSFC#&#&#51425301#&#&#21374021#&#&#51673096#&#&#U1601214 State Grid Corporation of science and technology projects Science and Technology Project of SGCC and The Research Foundation of Education Bureau of Hunan Province, China#&#&#15A091

机构署名：

本校为第一且通讯机构

院系归属：

理学院

摘要：

AbstractFor the first time, a three‐dimensional (3D) volume calculation model based on total electrostatic potential analysis and density functional calculations is applied to study the volume differences between hydrated multivalent vanadium ions (V2+, V3+, VO2+, and ) and charge‐balancing ions (H3O+, and ) encountered in the electrolyte solutions of vanadium redox flow batteries (VRBs). The calculated results indicate that radii of all charge‐balancing ions are less than 3.01 Å and of all hydrated multivalent vanadium ions are greate...

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Theoretical Investigation into Suitable Pore Sizes of Membranes for Vanadium Redox Flow Batteries

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