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Efficient charge transfer in aluminum-cobalt layered double hydroxide derived from Co-ZIF for enhanced catalytic degradation of tetracycline through peroxymonosulfate activation

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成果类型:
期刊论文
作者:
Cao, Jiao;Sun, Saiwu;Li, Xin;Yang, Zhaohui*;Xiong, Weiping;...
通讯作者:
Yang, Zhaohui
作者机构:
[Yang, Zhaohui; Cao, Jiao; Jia, Meiying; Zhang, Yanru; Wu, You; Sun, Saiwu; Xiong, Weiping; Zhou, Chengyun; Li, Xin] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
[Yang, Zhaohui; Cao, Jiao; Jia, Meiying; Zhang, Yanru; Wu, You; Sun, Saiwu; Xiong, Weiping; Zhou, Chengyun; Li, Xin] Hunan Univ, Minist Educ, Key Lab Environm Biol & Pollut Control, Changsha 410082, Peoples R China.
[Zhou, Yaoyu] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.
通讯机构:
[Yang, Zhaohui] H
Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
语种:
英文
关键词:
Actual wastewater;Aluminum-cobalt layered double hydroxide (AlCo-LDH);Cobalt zeolitic imidazolate framework (Co-ZIF);PMS activation;Tetracycline (TC)
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2020
卷:
382
页码:
122802
基金类别:
The obtained samples were initially investigated by SEM and XRD analysis. As shown in Fig. 1a and b, the Co-ZIF crystals exhibited a homogeneous hexagonal sheet morphology with a size of around 3.3 µm × 0.9 µm and a thickness of around 180 nm. The Co-ZIF crystals with a smooth surface and two-dimensional morphology were useful as in-situ etching for fabrication of porous MOFs derivatives. The as-obtained Co-ZIF showed high crystallinity and purity and the XRD pattern (Fig. 2a) matched well with
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院系归属:
资源环境学院
摘要:
In consideration of the complex synthesis of layered double hydroxides (LDHs), a simple and efficient strategy was needed to design and fabricate LDHs with high performance. In this study, aluminum-cobalt layered double hydroxide (AlCo-LDH) with uniformly distributed component was synthesized by in-situ etching of cobalt zeolitic imidazolate framework (Co-ZIF) at room temperature. The obtained AlCo-LDH showed high catalysis performance of tetracycline (TC) degradation via the activation of peroxymonosulfate (PMS). The removal efficiency can rea...

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