Lithiation-Derived Repellent toward Lithium Anode Safeguard in Quasi-solid Batteries

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成果类型：

期刊论文

作者：

Zeng, Xian-Xiang;Yin, Ya-Xia;Shi, Yang;Zhang, Xu-Dong;Yao, Hu-Rong;...

通讯作者：

Guo, Yu-Guo;Wu, Xiong-Wei

作者机构：

[Shi, Yang; Zhang, Xu-Dong; Yao, Hu-Rong; Zeng, Xian-Xiang; Yin, Ya-Xia; Wen, Rui; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.

[Wu, Xiong-Wei; Zeng, Xian-Xiang] Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

[Shi, Yang; Zhang, Xu-Dong; Yao, Hu-Rong; Zeng, Xian-Xiang; Yin, Ya-Xia; Wen, Rui; Guo, Yu-Guo] Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China.

通讯机构：

[Guo, Yu-Guo] C

[Wu, Xiong-Wei] H

[Guo, Yu-Guo] U

Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.

Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

语种：

英文

关键词：

interfacial repellent;ion transport;lithiation;lithium anode;quasi-solid batteries

期刊：

Chem

ISSN：

2451-9308

年：

2018

卷：

期：

页码：

298-307

DOI：

10.1016/j.chempr.2017.12.003

基金类别：

This work was supported by the Ministry of Science and Technology of the People's Republic of China (Grant grant Nono. 2016YFA0202500), the National Natural Science Foundation of China (Grant grant Nosnos. 21773264 and U1301244), and the “Strategic Priority Research Program” of the Chinese Academy of Sciences (Grant grant Nono. XDA09010300).

机构署名：

本校为通讯机构

院系归属：

理学院

摘要：

The aspiration of employing metallic lithium (Li) as the anode is impeded by Li dendrites and unwanted redox shuttles in liquid electrolytes. In this study, a repellent used to safeguard the Li anode was demonstrated during the lithiation of a nanosized AlPO4 additive in an infiltrated quasi-solid electrolyte (i-QSE) containing a concentrated electrolyte in a poly(tri-acrylate) network. As a result of the infiltrated structure, the ion transfer number of i-QSE attained 0.79, and the activation energy was only 0.12 eV. Compared with the control ...

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Lithiation-Derived Repellent toward Lithium Anode Safeguard in Quasi-solid Batteries

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