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Single-Atom Catalysts for Hydrogen Generation: Rational Design, Recent Advances, and Perspectives

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成果类型:
期刊论文
作者:
Zhang, Chenyu;Wang, Hou;Yu, Hanbo;Yi, Kaixin;Zhang, Wei;...
通讯作者:
Huang, Jinhui(huangjinhui@hnu.edu.cn);Zeng, Guangming(zgming@hnu.edu.cn);Deng, Yaocheng(dengyaocheng@hunau.edu.cn)
作者机构:
[Zeng, Guangming; Yuan, Xingzhong; Yi, Kaixin; Zhang, Wei; Wang, Hou; Yu, Hanbo; Huang, Jinhui; Zhang, Chenyu] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
[Deng, Yaocheng] Hunan Agr Univ, Coll Resources & Environm, Changsha 410082, Hunan, Peoples R China.
通讯机构:
[Jinhui Huang; Yaocheng Deng; Guangming Zeng] C
College of Resources and Environment, Hunan Agricultural University, Changsha, 410082 P. R. China<&wdkj&>College of Environmental Science and Engineering, Hunan University, Changsha, 410082 P. R. China
语种:
英文
关键词:
active site immobilization;electro-/photo-chemical hydrogen evolution;single-atom catalysts;structure–performance relationship;surface chemistry
期刊:
Advanced Energy Materials
ISSN:
1614-6832
年:
2022
卷:
12
期:
27
页码:
2200875-
基金类别:
C.Z. and H.W. contributed equally to this work. This work was supported by the National Natural Science Foundation of China (51909089, 22178091, 21776066, 51739004, and 51578222), Natural Science Foundation of Hunan Province, China (2020JJ5252), and China Postdoctoral Science Foundation (2019M662781).
机构署名:
本校为其他机构
院系归属:
资源环境学院
摘要:
Hydrogen is widely believed to be a promising fuel to solve the global energy crisis and environmental issues. The catalytic system represented by metal-supported catalysts is an important process of upgrading the hydrogen source in industry. Single-atom catalysts (SACs), which inherit the advantages of homogeneous and heterogeneous catalysts, provide a broad prospect for low-cost H2 production technology. This review focuses on the potential mechanisms in the rational design of SACs, including active sites, coordination configuration, mass loa...

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