A kind of Fe-Al bimetallic adsorbent was prepared and compared with other three kinds of adsorbent, including the acid-modified activated-carbon,ceramsite and hydrotalcite-like compound, for investigating their effects on removal of As(Ⅲ) from As-containing wastewater. Results showed that Fe-Al bimetallic material had a better effect of As(Ⅲ) adsorption than other 3 adsorbents, with an adsorption efficiency over 89%. It is found the As(Ⅲ) adsorption by Fe-Al bimetallic material conforms to Langmuir isotherm model and Freundlich isotherm mode...