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Recycled Tandem Catalysts Promising Ultralow Overpotential Li-CO₂ Batteries

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成果类型：

期刊论文

作者：

Lu, Bingyi;Min, Zhiwen;Xiao, Xiao;Wang, Boran;Chen, Biao;...

通讯作者：

Zhou, GM;Yang, JL;Sun, YM

作者机构：

[Xiao, Xiao; Lu, Bingyi; Wang, Boran; Mao, Rui; Liu, Yingqi; Zhou, Guangmin; Lu, Gongxun; Song, Yanze] Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China.

[Xiao, Xiao; Lu, Bingyi; Wang, Boran; Mao, Rui; Liu, Yingqi; Zhou, Guangmin; Lu, Gongxun; Song, Yanze] Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China.

[Yang, JL; Lu, Bingyi; Yang, Jinlong] Shenzhen Univ, Coll Mat Sci & Engn, Guangdong Res Ctr Interfacial Engn Funct Mat, Shenzhen Key Lab Energy Electrocatalyt Mat, Shenzhen 518060, Peoples R China.

[Min, Zhiwen; Sun, YM; Sun, Yuanmiao] Chinese Acad Sci, Fac Mat Sci & Energy Engn, Shenzhen Inst Adv Technol, Inst Technol Carbon Neutral, Shenzhen 518055, Peoples R China.

[Chen, Biao] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300350, Peoples R China.

通讯机构：

[Yang, JL ] S

[Sun, YM ] C

[Zhou, GM ] T

Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Peoples R China.

Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China.

语种：

英文

关键词：

bidirectional catalysts;in-built electric fields;Li-CO2 batteries;overpotential;spent lithium-ion batteries

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2024

卷：

期：

页码：

e2309264

DOI：

10.1002/adma.202309264

基金类别：

Natural Science Foundation of Guangdong Province; National Key Research and Development Program of China [2019YFA0705700]; National Natural Science Foundation of China [52172217]; Guangdong Innovative and Entrepreneurial Research Team Program [2021ZT09L197]; Shenzhen Stabilization Support Program [WDZC20200824091903001]; Shenzhen Science and Technology Program [JCYJ20210324120400002]; Interdisciplinary Research and Innovation Fund of Tsinghua Shenzhen International Graduate School; Science and Technology Innovation Program of Hunan Province [2023RC3154]; Testing Technology Center of Materials and Devices of Tsinghua Shenzhen International Graduate School; [2021A1515010144]

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摘要：

Lithium-carbon dioxide (Li-CO2) batteries are regarded as a prospective technology to relieve the pressure of greenhouse emissions but are confronted with sluggish CO2 redox kinetics and low energy efficiency. Developing highly efficient and low-cost catalysts to boost bidirectional activities is craved but remains a huge challenge. Herein, derived from the spent lithium-ion batteries, a tandem catalyst is subtly synthesized and significantly accelerates the CO2 reduction and evolution reactions (CO2RR and CO2ER) kinetics with an in-built electric field (BEF). Combining with the theoretical ca...

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