期刊论文

Yang, JL;Zhou, GM

英文

Advanced Materials

0935-9648

2024

36

1

2308889-

10.1002/adma.202308889

The authors appreciate support from the National Key Research and Development Program of China (2019YFA0705700), the National Natural Science Foundation of China (No. 52172217), the Natural Science Foundation of Guangdong Province (2021A1515010144), the Gu [2019YFA0705700]; National Key Research and Development Program of China [52172217]; National Natural Science Foundation of China [2021A1515010144]; Natural Science Foundation of Guangdong Province [2021ZT09L197]; Guangdong Innovative and Entrepreneurial Research Team Program [WDZC20200824091903001]; Shenzhen Stabilization Support Program [JCYJ20210324120400002]; Shenzhen Science and Technology Program; Interdisciplinary Research and Innovation Fund of Tsinghua Shenzhen International Graduate School [2023RC3154]; Science and Technology Innovation Program of Hunan Province; Testing Technology Center of Materials and Devices of Tsinghua Shenzhen International Graduate School

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Abstract Li‐CO2 batteries have aroused great interest in the context of carbon neutralization, but their practicability is severely hindered by the sluggish CO2 redox reaction kinetics at the cathode, which brings about formidable challenges such as high overpotential and low Coulombic efficiency. For the complex multi‐electron transfer process, the design of catalysts at the molecular or atomic level and the understanding of the relationship between electron state and performance are essential for the CO2 redox. However, little attention has...