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Insights into the oxidation of organic contaminants by iron nanoparticles encapsulated within boron and nitrogen co-doped carbon nanoshell: Catalyzed Fenton-like reaction at natural pH

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成果类型:
期刊论文
作者:
Zhou, Hao;Wu, Shikang;Zhou, Yaoyu*;Yang, Yuan;Zhang, Jiachao;...
通讯作者:
Zhou, Yaoyu;Tsang, Daniel C. W.
作者机构:
[Zhou, Hao; Yang, Yuan; Wu, Shikang; Zhou, Yaoyu; Zhang, Jiachao; Luo, Lin] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Hunan, Peoples R China.
[Zhou, Hao] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China.
[Zhou, Hao] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
[Wang, Shaobin; Duan, Xiaoguang] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia.
[Wang, Lei] Univ Sheffield, Dept Mat Sci & Engn, Sir Robert Hadfield Bldg,Mappin St, Sheffield S1 3JD, S Yorkshire, England.
通讯机构:
[Zhou, Yaoyu; Tsang, Daniel C. W.] H
Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Hunan, Peoples R China.
Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hung Hom, Kowloon, Hong Kong, Peoples R China.
语种:
英文
关键词:
Iron-based nanomaterials;Potassium monopersulfate;Fenton-like reaction;Antibiotics degradation;Green/sustainable remediation;Environmental catalysts
期刊:
Environment International
ISSN:
0160-4120
年:
2019
卷:
128
页码:
77-88
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51709103]; Natural Science Foundation of Hunan Province, ChinaNatural Science Foundation of Hunan Province [2018JJ3242]; China Postdoctoral Science FoundationChina Postdoctoral Science Foundation [2018M630901]; Hong Kong Scholars Program [XJ2018029]; Hong Kong Research Grants CouncilHong Kong Research Grants Council [E-PolyU503/17]
机构署名:
本校为第一且通讯机构
院系归属:
资源环境学院
摘要:
Iron nanoparticles encapsulated within boron and nitrogen co-doped carbon nanoshell (B/N-C@Fe) were synthesized through a novel and green pyrolysis process using melamine, boric acid, and ferric nitrate as the precursors. The surface morphology, structure, and composition of the B/N-C@Fe materials were thoroughly investigated. The materials were employed as novel catalysts for the activation of potassium monopersulfate triple salt (PMS) for the degradation of levofloxacin (LFX). Linear sweep voltammograms and quenching experiments were used to ...

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