N-doped carbon carriers loaded with NiX (X = Fe, Co, Cu): Catalytic synergistic pyrolysis of herbal residues and polypropylene to generate three-phase products and carbon nanotubes

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成果类型：

期刊论文

作者：

Chen, Zhaoguang;Xie, Yu;Yi, Cheng;Yao, Lingling;Li, Bo;...

通讯作者：

Zhi Zhou

作者机构：

College of Agronomy, Hunan Agricultural University, Changsha 410128, China

[Xie, Yu; Yi, Cheng] School of Chemistry and Materials Science, Hunan Agricultural University, Changsha 410128, China

Hunan Engineering Research Center for Biochar, Hunan Agricultural University, Changsha 410128, China

National Center of Technology Innovation for Saline-Alkali Tolerant Rice, Changsha 410125, China

[Chen, Zhaoguang; Yao, Lingling; Li, Bo] School of Chemistry and Materials Science, Hunan Agricultural University, Changsha 410128, China<&wdkj&>Hunan Engineering Research Center for Biochar, Hunan Agricultural University, Changsha 410128, China

通讯机构：

[Zhi Zhou] S

School of Chemistry and Materials Science, Hunan Agricultural University, Changsha 410128, China<&wdkj&>Hunan Engineering Research Center for Biochar, Hunan Agricultural University, Changsha 410128, China<&wdkj&>National Center of Technology Innovation for Saline-Alkali Tolerant Rice, Changsha 410125, China

语种：

英文

期刊：

Fuel

ISSN：

0016-2361

年：

2025

卷：

381

页码：

133548

DOI：

10.1016/j.fuel.2024.133548

基金类别：

CRediT authorship contribution statement Zhaoguang Chen: Writing – original draft, Methodology, Conceptualization. Yu Xie: Software, Resources. Cheng Yi: Visualization, Investigation. Lingling Yao: Formal analysis, Data curation. Bo Li: Validation. Zhi Zhou: Supervision, Project administration. Wei Luo: Writing – review & editing, acquisition.

机构署名：

本校为第一且通讯机构

院系归属：

农学院

摘要：

Catalytic pyrolysis can transform organic solid waste into high-quality pyrolysis products, in which N-doped biochar is an efficient and economical catalyst. Herein, N-doped activated carbon (NAC) and modified biochar (NZC) loaded with bimetal NiX (X = Fe, Co, Cu) were used to catalyze the pyrolysis of Chinese medicinal drug residue and polypropylene in a two-stage reaction system to prepare three-phase products and carbon nanotubes. This indicates that the metal/NAC group catalysts possess a larger S BET , whereas the metal/NZC group has better thermal stability. Under NiCo/NZC catalysis, the...

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N-doped carbon carriers loaded with NiX (X = Fe, Co, Cu): Catalytic synergistic pyrolysis of herbal residues and polypropylene to generate three-phase products and carbon nanotubes

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