Experimental and theoretical insights into kinetics and mechanisms of hydroxyl and sulfate radicals-mediated degradation of sulfamethoxazole: Similarities and differences

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成果类型：

期刊论文

作者：

Gao, Lingwei;Mao, Qiming;Luo, Shuang*;Cao, Linying;Xie, Xiande;...

通讯作者：

Luo, Shuang;Wei, Zongsu

作者机构：

[Xie, Xiande; Mao, Qiming; Yang, Yuan; Cao, Linying; Luo, Shuang; Gao, Lingwei] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.

[Gao, Lingwei] Cent South Univ, Sch Met & Environm, Inst Environm Engn, Changsha 410083, Peoples R China.

[Deng, Yunfeng] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.

[Deng, Yunfeng] Tianjin Univ, Tianjin Key Lab Mol Optoelect Sci, Tianjin 300072, Peoples R China.

[Wei, Zongsu] Aarhus Univ, Ctr Water Technol WATEC, Dept Engn, Hangovej 2, DK-8200 Aarhus N, Denmark.

通讯机构：

[Luo, Shuang] H

[Wei, Zongsu] A

Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.

Aarhus Univ, Ctr Water Technol WATEC, Dept Engn, Hangovej 2, DK-8200 Aarhus N, Denmark.

语种：

英文

关键词：

Advanced oxidation;Hydroxyl radical;Sulfamethoxazole;Sulfate radical;Theoretical calculation

期刊：

Environmental Pollution

ISSN：

0269-7491

年：

2020

卷：

259

页码：

113795

DOI：

10.1016/j.envpol.2019.113795

基金类别：

Acknowledgments from National Natural Science Foundation of China of China (21806035, 21806003), National Nature Science Foundation of Hunan province (2019JJ50226), National Key R&D Projects of China (2016YFC0403002), Hunan Provincial Key R&D (2018WK4007, 2019SK2281), and Aarhus University Centre for Water Technology (AU-WATEC) Start-Up Fund from the Poul Due Jensen Foundation is gratefully acknowledged.

机构署名：

本校为第一且通讯机构

院系归属：

资源环境学院

摘要：

This study provides insights into the similarities and differences of degradation reactions by •OH/[Formula presented] at the molecular level for improved antibiotics removal. © 2019 Elsevier LtdHydroxyl radical (•OH)- and sulfate radical ([Formula presented])-based advanced oxidation technologies (AOTs) have been proven an effective method to remove antibiotics in wastewater treatment plants (WWTPs). This study aims to gain insights into kinetics and mechanisms of neutral sulfamethoxazole (SMX) degradation, a representative antibiotic, by •...

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Experimental and theoretical insights into kinetics and mechanisms of hydroxyl and sulfate radicals-mediated degradation of sulfamethoxazole: Similarities and differences

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