Efficient Neutral Nitrate-to-Ammonia Electrosynthesis Using Synergistic Ru-Based Nanoalloys on Nitrogen-Doped Carbon

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成果类型：

期刊论文

作者：

Huang, Lisi;Zhang, Pingzhi;Ge, Xin;Wang, Bingyu;Yuan, Jili;...

通讯作者：

Yuan, JL;Li, W;Wang, L;Zhang, J

作者机构：

[Yuan, Jili; Huang, Lisi; Ge, Xin; Wang, Bingyu] Guizhou Univ, Coll Mat & Met, Dept Polymer Mat & Engn, Guiyang 550025, Peoples R China.

[Zhang, Pingzhi; Li, Wei] Hunan Agr Univ, Sch Chem & Mat Sci, Changsha 410128, Peoples R China.

[Wang, Liang] Shanghai Univ, Inst Nanochem & Nanobiol, Sch Environm & Chem Engn, 99 Shangda Rd, Shanghai 200444, Peoples R China.

[Zhang, Baohua] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, 99 Shangda Rd, Shanghai 200444, Peoples R China.

[Huang, Lisi; Zhang, Jian] Guizhou Univ, State Key Lab Green Pesticide, Ctr R&D Fine Chem, Guiyang 550025, Peoples R China.

通讯机构：

[Yuan, JL ; Zhang, J ] G

[Li, W ] H

[Wang, L ] S

Guizhou Univ, Coll Mat & Met, Dept Polymer Mat & Engn, Guiyang 550025, Peoples R China.

Hunan Agr Univ, Sch Chem & Mat Sci, Changsha 410128, Peoples R China.

语种：

英文

关键词：

Nanoalloys;Neutral NH3 electrosynthesis;Porous nitrogen-doped carbon;Selective etching;Synergic effect

期刊：

纳微快报(英文)

ISSN：

2311-6706

年：

2026

卷：

期：

页码：

1-14

DOI：

10.1007/s40820-025-01896-w

基金类别：

National Natural Science Foundation of China [22466010]; Guizhou Provincial Basic Research Program (Natural Science) [ZK[2023]47, ZD[2025]075]; Innovation and Entrepreneurship Project for overseas Talents in Guizhou Province [[2022]02]; Specific Natural Science Foundation of Guizhou University [X202207]; The national undergraduate innovation and entrepreneurship training program [gzugc2023006, gzusc2024012]; SRT project of Guizhou university [2023SRT029, 2023SRT024]; Shanghai Technical Service Center of Science and Engineering Computing, Shanghai University

机构署名：

本校为通讯机构

摘要：

Electrocatalytic nitrate reduction reaction (NO(3)RR) represents a sustainable and environmentally benign route for ammonia (NH(3)) synthesis. However, NO(3)RR is still limited by the competition from hydrogen evolution reaction (HER) and the high energy barrier in the hydrogenation step of nitrogen-containing intermediates. Here, we report a selective etching strategy to construct RuM nanoalloys (M = Fe, Co, Ni, Cu) uniformly dispersed on porous nitrogen-doped carbon substrates for efficient neutral NH(3) electrosynthesis. Density functional...

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Efficient Neutral Nitrate-to-Ammonia Electrosynthesis Using Synergistic Ru-Based Nanoalloys on Nitrogen-Doped Carbon

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