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Cr-Mn bimetallic functionalized USY zeolite monolithic catalyst for direct production of 2, 5-Furandicarboxylic acid from raw biomass

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成果类型:
期刊论文
作者:
Chai, Youzheng;Bai, Ma;Chen, Anwei*;Yuan, Jiayi;Peng, Cheng;...
通讯作者:
Chen, Anwei
作者机构:
[Yan, Binghua; Qin, Pufeng; Yuan, Jiayi; Peng, Cheng; Chen, Anwei; Zhao, Danyao; Chai, Youzheng; Bai, Ma] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.
通讯机构:
[Chen, Anwei] H
Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.
语种:
英文
关键词:
Biomass;Biorefining;5-furandicarboxylic acid;Cr-Mn;Monolithic catalyst
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2022
卷:
429
页码:
132173
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51879105, 51808215]; Hunan Provincial Natural Science Foundation of ChinaNatural Science Foundation of Hunan Province [2019JJ40128, 2019JJ50253]
机构署名:
本校为第一且通讯机构
院系归属:
资源环境学院
摘要:
The production of biomass-based 2, 5-furandicarboxylic acid occupies a vital position in biorefining. Here, Cr-Mn bimetallic supported Ultra-stabilized Y (USY) zeolite monolithic catalyst was prepared by the impregnation method, which aimed to direct catalyze the production of 2, 5-Furandicarboxylic acid (FDCA) from raw material biomass. The yield of FDCA could reach 67% with optimum conditions, and the catalyst has stable recyclability. Characterization analysis showed that the coordination of Cr and Mn increased oxygen mobility. The combinati...

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