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Ultrafast photodegradation of nitenpyram by Ag/Ag3PO4/Zn–Al LDH composites activated by persulfate system: Removal efficiency, degradation pathway and reaction mechanism

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成果类型:
期刊论文
作者:
Zheng, Jiangfu;Li, Wenbo;Tang, Rongdi;Xiong, Sheng;Gong, Daoxin*;...
通讯作者:
Gong, Daoxin;Deng, YC
作者机构:
[Tang, Rongdi; Deng, Yaocheng; Li, Ling; Gong, Daoxin; Su, Long; Gong, DX; Zhou, Zhanpeng; Yang, Lihua; Xiong, Sheng; Zheng, Jiangfu] Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.
[Li, Wenbo] Hunan Prov Environm Protect Engn Ctr Organ Pollut, Changsha 410001, Hunan, Peoples R China.
通讯机构:
[Gong, DX; Deng, YC ] H
Hunan Agr Univ, Coll Resources & Environm, Changsha 410128, Peoples R China.
语种:
英文
关键词:
Catalytic degradation;Layered double hydroxides;Nitenpyram;Persulfate activation;Silver phosphate
期刊:
Chemosphere
ISSN:
0045-6535
年:
2022
卷:
292
页码:
133431
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51909089]; Natural Science Foundation of Hunan Province, ChinaNatural Science Foundation of Hunan Province [2020JJ5252]; China Postdoctoral Science FoundationChina Postdoctoral Science Foundation [2019M662781]; Scientific Research Project of Hunan Provincial Department of Education, China [19C0919]; Science Foundation for Young Scholars of Hunan Agricultural University [19QN35]; Hunan Provincial Innovation Foundation for Postgraduate [CX20200663]
机构署名:
本校为第一且通讯机构
院系归属:
资源环境学院
摘要:
In this study, an investigation is conducted into the degradation of nitenpyram (NTP) using highly efficient APMMO/PDS/Vis system. As photocatalysts, silver phosphate (AP) and calcined Zn-Al layered double hydroxides (MMO) exhibit high efficiency in achieving charge separation. Besides, the injection of electrons into peroxydisulfate (PDS) from the APMMO can contribute to obtaining the species in the active state with higher efficiency. Based on the APMMO/PDS/Vis system, 50 mg/L of nitenpyram (NTP, 50 mL) can be completely removed in 60 min using 0.8 g/L photocatalyst and 0.2 g/L PDS under the...

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