Rhodium-catalyzed oxidative decarbonylative Heck-type coupling of aromatic aldehydes with terminal alkenes

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成果类型：

期刊论文

作者：

Kang, Lei;Zhang, Feng;Ding, Lin-Ting;Yang, Luo*

通讯作者：

Yang, Luo

作者机构：

[Ding, Lin-Ting; Kang, Lei; Yang, Luo] Xiangtan Univ, Coll Chem, Minist Educ, Key Lab Environm Friendly Chem & Applicat, Xiangtan 411105, Hunan, Peoples R China.

[Zhang, Feng] Hunan Agr Univ, Coll Sci, Changsha 410128, Hunan, Peoples R China.

通讯机构：

[Yang, Luo] X

Xiangtan Univ, Coll Chem, Minist Educ, Key Lab Environm Friendly Chem & Applicat, Xiangtan 411105, Hunan, Peoples R China.

语种：

英文

期刊：

RSC Advances

ISSN：

2046-2069

年：

2015

卷：

期：

122

页码：

100452-100456

DOI：

10.1039/c5ra21610a

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21202138, 21302051]; Xiangtan University "Academic Leader Program" [11QDZ20]; New Teachers' Fund for Doctor Stations, Ministry of Education [20124301120007]; Hunan Provincial Natural Science FoundationNatural Science Foundation of Hunan Province [13JJ4047]; Hunan Provincial Excellent Young Scientist Foundation [13B114]

机构署名：

本校为其他机构

院系归属：

理学院

摘要：

A rhodium-catalyzed oxidative decarbonylative Heck-type coupling of aromatic aldehydes with terminal alkenes to afford 1,2-disubstituted alkenes with good regio- and E-selectivity is developed. This reaction employs readily available aromatic aldehydes as the aryl electrophile counterpart and relies on selected acyl chloride as the crucial additive to activate the rhodium catalyst pre...

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Rhodium-catalyzed oxidative decarbonylative Heck-type coupling of aromatic aldehydes with terminal alkenes

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