Preferred Orientation Deposition via Multifunctional Gel Electrolyte with Molecular Anchor Enabling Highly Reversible Zn Anode

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成果类型：

期刊论文

作者：

Xu, Yu-Ting;Dai, Sheng-Jia;Gong, Ming-Jun;Zhang, Ji-Zun;Xu, Hai;...

通讯作者：

Wang, XF;Zeng, XX

作者机构：

[Xu, Yu-Ting; Li, Aijun; Wang, Xiao-Feng; Zhang, Ji-Zun] Jilin Univ, Coll Phys, Key Lab Phys & Technol Adv Batteries, Minist Educ, Changchun 130012, Peoples R China.

[Dai, Sheng-Jia; Wu, Xiong-Wei; Gong, Ming-Jun; Zeng, Xian-Xiang] Hunan Agr Univ, Sch Chem & Mat Sci, Changsha 410128, Hunan, Peoples R China.

[Xu, Hai] Jilin Univ, Coll Chem, Changchun 130012, Peoples R China.

[Sasaki, Shin-ichi] Ritsumeikan Univ, Grad Sch Life Sci, Kusatsu, Shiga 5258577, Japan.

通讯机构：

[Zeng, XX ] H

[Wang, XF ] J

Jilin Univ, Coll Phys, Key Lab Phys & Technol Adv Batteries, Minist Educ, Changchun 130012, Peoples R China.

Hunan Agr Univ, Sch Chem & Mat Sci, Changsha 410128, Hunan, Peoples R China.

语种：

英文

关键词：

aqueous zinc-ion batteries;dendrite-free Zn anodes;gel electrolytes;hydrogen evolution reaction;preferred orientation

期刊：

Small

ISSN：

1613-6810

年：

2024

卷：

期：

页码：

e2304463

DOI：

10.1002/smll.202304463

基金类别：

National Natural Science Foundation of China; Basic Science Center Project of the National Key Research and Development Program of China [2021YFB2400400]; Japan Society for the Promotion of Science (JSPS) KAKENHI [22k05260]; [11974129]; [62274075]; [51803054]

机构署名：

本校为通讯机构

摘要：

A gel electrolyte with molecular anchors is synthesized. It reduces the activity of H2O by anchoring them through ternary hydrogen bonds, which effectively inhibits hydrogen evolution reaction. Furthermore, multiple charged groups of the gel electrolyte induce the deposition of Zn2+ in an orderly manner and promote the directional deposition of Zn2+ on the Zn (002) plane, obtaining a highly reversible dendrite‐free anode. Abstract The high activity of water molecules results in a series of awful parasitic reaction, which seriously impede the d...

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Preferred Orientation Deposition via Multifunctional Gel Electrolyte with Molecular Anchor Enabling Highly Reversible Zn Anode

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