The Mg/Al layered double hydroxide (Mg/Al-LDH) intercalated with the [Formula: see text] (MoS4-LDH) impregnated into poly(acrylamide-co-sodium acrylate) (PP) was synthesized as layered double hydroxides-PP (LDHS-PP), whose characterization, adsorption properties and mechanisms were investigated. The maximum adsorption capacity (qm) for Cd(II) was approximately 2789.58 mg/g by 1% LDHS-PP, while it was approximately 1893.09 mg/g by PP, which indicated that the MoS4-LDH greatly improved the Cd(II) uptake for PP in aqueous solution. In strongly acidic conditions ( approximately pH 3.0), there was ...