期刊论文

Liang, Yun

英文

JOURNAL OF ORGANIC CHEMISTRY

0022-3263

2014

79

22

11264-11269

10.1021/jo502098b

Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21072054]; Ministry of Education of ChinaMinistry of Education, China [20094306120003, 213027A]; Training Program Foundation for the Young Talents by Hunan Normal University [ET21003]; Hunan Provincial Natural Science FoundationNatural Science Foundation of Hunan Province [12JJ2009]; Scientific Research Fund of Hunan Provincial Education DepartmentHunan Provincial Education Department [12A095]; Aid Program for Science and Technology Innovative Research Team in Higher Educational Institutions of Hunan Province

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A metal-free decarboxylative amination of 4-(ethoxycarbonyl)-2,3-allenols by TsNCO via base-induced aza-Michael addition/elimination has been developed. A variety of substituted N-tosyl 1,3-dien-2-yl amines were obtained in good yields and excellent regio- and stereoselectivity. Moreover, this transformation could be ap...