Unveiling the Role of Heteroatom Gradient-Distributed Carbon Fibers for Vanadium Redox Flow Batteries with Long Service Life

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成果类型：

期刊论文

作者：

Wu, Xiong-Wei;Deng, Qi*;Peng, Chang;Zeng, Xian-Xiang;Wu, An-Jun;...

通讯作者：

Deng, Qi;Lu, Xiang-Yang;Guo, Yu-Guo

作者机构：

[Wu, An-Jun; Ma, Qiang; Wu, Xiong-Wei; Peng, Chang; Deng, Q; Lu, Xiang-Yang; Deng, Qi; Zeng, Xian-Xiang; Zhou, Chun-Jiao] Hunan Agr Univ, Coll Sci, Coll Biosci & Biotechnol, Changsha 410128, Hunan, Peoples R China.

[Yin, Ya-Xia; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, CAS Key Lab Mol Nanostruct & Nanotechnol, CAS Res Educ Ctr Excellence Mol Sci,BNLMS, Beijing 100190, Peoples R China.

[Yin, Ya-Xia; Guo, Yu-Guo] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.

通讯机构：

[Deng, Q; Lu, XY] H

[Guo, Yu-Guo] C

[Guo, Yu-Guo] U

Hunan Agr Univ, Coll Sci, Coll Biosci & Biotechnol, Changsha 410128, Hunan, Peoples R China.

Chinese Acad Sci, Inst Chem, CAS Key Lab Mol Nanostruct & Nanotechnol, CAS Res Educ Ctr Excellence Mol Sci,BNLMS, Beijing 100190, Peoples R China.

语种：

英文

关键词：

vanadium redox flow batteries;electrocatalysis;carbon fibers;heteroatoms gradient distribution;long service life

期刊：

ACS Applied Materials & Interfaces

ISSN：

1944-8244

年：

2019

卷：

期：

页码：

11451-11458

DOI：

10.1021/acsami.8b22521

基金类别：

This work was financially supported by the Basic Science Center Project of Natural Science Foundation of China (Grant no. 51788104), the National Key R&D Program of China (Grant no. 2016YFA0202500), the “Transformational Technologies for Clean Energy and Demonstration”, Strategic Priority Research Program of the Chinese Academy of Sciences (Grant no. XDA21070300), the Double First-Class Construction Project of Hunan Agricultural University (Grant no. SYL201802002, SYL201802008), and the Scientific Research Fund of Hunan Provincial Education Department (Grant no. 15 K058).

机构署名：

本校为第一且通讯机构

院系归属：

理学院

生物科学技术学院

摘要：

The fundamental understanding of electrocatalytic reaction process is anticipated to guide electrode upgradation and acquirement of high-performance vanadium redox flow batteries (VRFBs). Herein, a carbon fiber prototype system with a heteroatom gradient distribution has been developed with enlarged interlayer spacing and a high graphitization that improve the electronic conductivity and accelerate the electrocatalytic reaction, and the mechanism by which gradient-distributed heteroatoms enhance vanadium redox reactions was elucidated with the ...

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Unveiling the Role of Heteroatom Gradient-Distributed Carbon Fibers for Vanadium Redox Flow Batteries with Long Service Life

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