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A theoretical study of the effect and mechanism of FeN3-doped biochar for greenhouse gas mitigation

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成果类型:
期刊论文
作者:
Wang, Hong-Rui;Zhou, Wen-Tao;Xiong, Rui;Zhong, Kang-Yu;He, Jing;...
通讯作者:
Zhi-Qiang Fu
作者机构:
[Long, Pan; Zhou, Wen-Tao; Xiong, Rui; Fu, Zhi-Qiang; Zhong, Kang-Yu; Wang, Hong-Rui; He, Jing] Hunan Agr Univ, Coll Agron, Changsha 410128, Peoples R China.
[Ma, Xin; Wu, Qing] Cent South Univ, Coll Chem & Chem Engn, Informat & Network Ctr, Changsha 410083, Peoples R China.
通讯机构:
[Zhi-Qiang Fu] C
College of Agronomy, Hunan Agricultural University, Changsha, People’s Republic of China
语种:
英文
关键词:
Modified biochar;Fe atoms sorbent;Greenhouse gas;First-principles calculation;Adsorption mechanism
期刊:
生物炭
ISSN:
2524-7972
年:
2023
卷:
5
期:
1
页码:
1-10
基金类别:
This work was supported by National Key Research and Development Programs (2022YFD2300305), the Natural Science Foundation of Hunan Province (2021JJ30319), Graduate Research Innovation Project of Hunan Agricultural University.
机构署名:
本校为第一机构
院系归属:
农学院
摘要:
Paddy fields are a major emission source of greenhouse gases (GHGs) [for instance, methane (CH4), nitrous oxide (N2O), and carbon dioxide (CO2)] among agricultural fields. Biochar has been deemed a potential candidate for the reduction of GHGs in paddy fields. However, there is no consistent conclusion that biochar can simultaneously reduce emissions of CH4, N2O, and CO2. Herein, we proposed the FeN3-doped biochar (FG) as an excellent material for GHGs restriction in paddy fields via the first-principles calculation. The computation results ind...

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